Establishment and Characteristics of An Anthropogenic Ammonia Emissions Inventory in Jiangsu Province from 2013 to 2017

HOU Xin-hong1 YU Xing-na1 SHEN Li1 ZHAO Rui-dong1 WANG Guo-zhen1 ZHANG Yu-xiu1

(1.Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters, Nanjing University of Information Science and Technology , Nanjing, China 210044)

【Abstract】According to the activity level data of various ammonia emission sources in Jiangsu Province, by a reasonable inventory calculation method and emission factor (EF), an ammonia emission inventory in Jiangsu Province from 2013 to 2017 was established, and the trend of anthropogenic emissions over these years was analyzed. The distribution characteristics of anthropogenic emissions and emission intensity in Jiangsu Province were analyzed using Arc GIS software. The results showed that the ammonia emissions in Jiangsu Province decreased from 624.84 kt in 2013 to 562.47 kt in 2017 with an average annual decreased rate of approximately 2.6%. Agricultural has always been the most important source of ammonia emissions in Jiangsu Province and accounted for 82.4% of the total ammonia emissions in 2017. Laying hens are the largest source of ammonia emissions from livestock and poultry sources, accounting for 49.3% of the ammonia emissions from livestock and poultry. The average ammonia emission intensity in Jiangsu Province was 5.3 t·km−2 in 2017. Yancheng and Xuzhou are two cities with the largest anthropogenic emission and emission intensity in Jiangsu Province. Zhenjiang City has the lowest ammonia emission and emission intensity.

【Keywords】 ammonia; emission factor; emission inventory; emission intensity; Jiangsu Province;

【DOI】

【Funds】 National Key Research and Development Project of China(2016YFC0203501) National Natural Science Foundation of China (41775154) Six Categories of Summit Talents of Jiangsu Province of China (JNHB-057) “Qinglan” Project Foundation of Jiangsu Province

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    References

    [1] Galloway J N, Dianwu Z, Thomson V E, et al. Nitrogen mobilization in the United States of America and the People’s Republic of China [J]. Atmospheric Environment, 1996, 30 (10–11): 1551–1561.

    [2] Battye W, Aneja V P, Roelle P A. Evaluation and improvement of ammonia emissions inventories [J]. Atmospheric Environment, 2003, 37 (27): 3873–3883.

    [3] Shen L, Yu X N, Xiang L. Estimation of ammonia emissions inventories in Jiangsu Province from 2006 to 2014 [J]. China Environmental Science, 2018, 38 (1): 26–34 (in Chinese with English abstract).

    [4] Sutton M A, Dragosits U, Tang Y S, et al. Ammonia emissions from non-agricultural sources in the UK [J]. Atmospheric Environment, 2000, 34 (6): 855–869.

    [5] Sun Q R, Wang M R. Ammonia emission and concentration in the atmosphere over China [J]. Scientia Atmospherica Sinica, 1997, 21 (5): 590–598 (in Chinese with English abstract).

    [6] Wang W X, Lu X F, Pang Y B, et al. Geographical distribution of NH3 emission intensities in China [J]. Acta Scientiae Circumstantiae, 1997, 17 (1): 2–7.

    [7] Wang C, Yin S S, Yu S J, et al. A 2013-based atmospheric ammonia emission inventory and its characteristic of spatial distribution in Henan Province [J]. Environmental Science, 2018, 39 (3): 1023–1030 (in Chinese with English abstract).

    [8] Dong Y Q, Chen C H, Huang C, et al. Anthropogenic emissions and distribution of ammonia over the Yangtze River Delta [J]. Acta Scientiae Circumstantiae, 2009, 29 (8): 1611–1617 (in Chinese with English abstract).

    [9] Yin S S, Zheng J Y, Zhang L J, et al. Anthropogenic ammonia emission inventory and characteristics in the Pearl River Delta Region [J]. Environmental Science, 2010, 31 (5): 1146–1151 (in Chinese with English abstract).

    [10] Yin S S. Study on Anthropogenic ammonia Emission Inventory in the Pearl River Delta and effects on source contribution to particulate matter formation [D]. Guangzhou: South China University of Technology, 2011 (in Chinese with English abstract).

    [11] Zhou J, Liu S H, Tan Y, et al. Anthropogenic ammonia emission inventory and its spatial distribution in Suzhou City [J]. Research of Environmental Sciences, 2016, 29 (8): 1137–1144 (in Chinese with English abstract).

    [12] Su H, Yan D J, Huang X M, et al. Inventory and characteristics of anthropogenic ammonia emission in Xi’an [J]. Environmental Science, 2016, 37 (11): 4117–4123 (in Chinese with English abstract).

    [13] Wang P. Estimation on anthropogenic emissions of ammonia in Nantong [J]. Environmental Science and Management, 2012, 37 (11): 25–28 (in Chinese with English abstract).

    [14] Kang Y M, Liu M X, Song Y, et al. High-resolution ammonia emissions inventories in China from 1980 to 2012 [J]. Atmospheric Chemistry and Physics, 2016, 16 (4): 2043–2058.

    [15] Ministry of Ecology and Environment of the People’s Republic of China. 大气氨源排放清单编制技术指南 (试行) [EB/OL]. http://www.mee.gov.cn/gkml/hbb/bgg/201408/W020140828351293771578.pdf, 2014-08=19 (in Chinese).

    [16] Jiangsu Provincial Bureau of Statistics, Bureau Zhejiang Survey Team of the National Bureau of Statistics of China. Jiangsu Statistical Yearbook 2014 [M]. Beijing: China Statistics Press, 2014 (in Chinese).

    [17] Jiangsu Provincial Bureau of Statistics, Bureau Zhejiang Survey Team of the National Bureau of Statistics of China. Jiangsu Statistical Yearbook 2015 [M]. Beijing: China Statistics Press, 2015 (in Chinese).

    [18] Jiangsu Provincial Bureau of Statistics, Bureau Zhejiang Survey Team of the National Bureau of Statistics of China. Jiangsu Statistical Yearbook 2016 [M]. Beijing: China Statistics Press, 2016 (in Chinese).

    [19] Jiangsu Provincial Bureau of Statistics, Bureau Zhejiang Survey Team of the National Bureau of Statistics of China. Jiangsu Statistical Yearbook 2017 [M]. Beijing: China Statistics Press, 2017 (in Chinese).

    [20] Jiangsu Provincial Bureau of Statistics, Bureau Zhejiang Survey Team of the National Bureau of Statistics of China. Jiangsu Statistical Yearbook 2018 [M]. Beijing: China Statistics Press, 2018 (in Chinese).

    [21] Department of Energy Statistics, National Bureau of Statistics of China. China Energy Statistical Yearbook 2013 [M]. Beijing: China Statistics Press, 2013 (in Chinese).

    [22] Department of Energy Statistics, National Bureau of Statistics of China. China Energy Statistical Yearbook 2014 [M]. Beijing: China Statistics Press, 2014 (in Chinese).

    [23] Department of Energy Statistics, National Bureau of Statistics of China. China Energy Statistical Yearbook 2015 [M]. Beijing: China Statistics Press, 2015 (in Chinese).

    [24] Department of Energy Statistics, National Bureau of Statistics of China. China Energy Statistical Yearbook 2016 [M]. Beijing: China Statistics Press, 2016 (in Chinese).

    [25] Department of Energy Statistics, National Bureau of Statistics of China. China Energy Statistical Yearbook 2017 [M]. Beijing: China Statistics Press, 2017 (in Chinese).

    [26] Ministry of Housing and Urban-Rural Development of the People’s Republic of China. China Urban Construction Statistical Yearbook 2011 [M]. Beijing: China Planning Press, 2011 (in Chinese).

    [27] Ministry of Housing and Urban-Rural Development of the People’s Republic of China. China Urban Construction Statistical Yearbook 2012 [M]. Beijing: China Planning Press, 2012 (in Chinese).

    [28] Ministry of Housing and Urban-Rural Development of the People’s Republic of China. China Urban Construction Statistical Yearbook 2013 [M]. Beijing: China Statistics Press, 2013 (in Chinese).

    [29] Ministry of Housing and Urban-Rural Development of the People’s Republic of China. China Urban Construction Statistical Yearbook 2014 [M]. Beijing: China Statistics Press, 2014 (in Chinese).

    [30] Ministry of Housing and Urban-Rural Development of the People’s Republic of China. China Urban Construction Statistical Yearbook 2015 [M]. Beijing: China Statistics Press, 2015 (in Chinese).

    [31] Buijsman E, Maas H F M, Asman W A H. Anthropogenic NH3 emissions in Europe [J]. Atmospheric Environment, 1987, 21 (5): 1009–1022.

    [32] Ryden J C, Whitehead D C, Lockyer D R, et al. Ammonia emission from grassland and livestock production systems in the UK [J]. Environmental Pollution, 1987, 48 (3): 173–184.

    [33] Yang Z P. Estimation of ammonia emissions from livestock in China based on mass-flow method and regional comparison [D]. Beijing: Peking University, 2008 (in Chinese with English abstract).

    [34] Liu B, Tong Y, Li A, et al. Study on ammonia emission inventory of livestock over Yangtze River Delta [J]. Journal of Ecology and Rural Environment, 2018, 34 (11): 1042–1049 (in Chinese with English abstract).

    [35] Shen X L. A highly resolved anthropogenic ammonia emission inventory in Guangdong Province and assessment of control strategies [D]. Guangzhou: South China University of Technology, 2014 (in Chinese with English abstract).

    [36] Deng M H, Yin B, Zhang S L, et al. Effects of rate and method of N application on ammonia volatilization in paddy fields [J]. Soils, 2006, 38 (3): 263–269 (in Chinese with English abstract).

    [37] Deng M J, Luo W B. Space-time evolution of China’s agricultural ammonia emission and emission reduction potential [J]. Chinese Journal of Eco-Agriculture, 2018, 26 (9): 1257–1268 (in Chinese with English abstract).

    [38] Dong W X, Xing J, Wang S X. Temporal and spatial distribution of anthropogenic ammonia emissions in China: 1994–2006 [J]. Environmental Science, 2010, 31 (7): 1457–1463 (in Chinese with English abstract).

    [39] Che W W. A highly resolved mobile source emission inventory in the Pearl River Delta and assessment of motor vehicle pollution control strategies [D]. Guangzhou: South China University of Technology, 2010 (in Chinese with English abstract).

    [40] Che W W, Zheng J Y, Zhong L J. Vehicle exhaust emission characteristics and contributions in the Pearl River Delta Region [J]. Research of Environmental Sciences, 2009, 22 (4): 456–461 (in Chinese with English abstract).

    [41] Wang S X, Zhang C Y. Spatial and temporal distribution of air pollutant emissions from open burning of crop residues in China [J]. Sciencepaper Online, 2008, 3 (5): 329–333 (in Chinese).

    [42] Zhang H F. A Laboratory study on emission characteristics of gaseous and particulate pollutants emitted from agricultural crop residue burning in China [D]. Shanghai: Fudan University, 2009 (in Chinese).

    [43] Department of Industry and Transport Statistics, National Bureau of Statistics of China. China Energy Statistical Yearbook 2005 [M]. Beijing: China Statistics Press, 2005 (in Chinese).

    [44] Department of Industry and Transport Statistics, National Bureau of Statistics of China. China Energy Statistical Yearbook 2006 [M]. Beijing: China Statistics Press, 2006 (in Chinese).

    [45] Department of Industry and Transport Statistics, National Bureau of Statistics of China. China Energy Statistical Yearbook 2007 [M]. Beijing: China Statistics Press, 2007 (in Chinese).

    [46] Bu M D, Zhang T. Assessment of methane production from domestic waste landfill in China [J]. Renewable Energy Resources, 2012, 30 (5): 89–94, 99 (in Chinese with English abstract).

    [47] Liu C L, Yang F. Nanjing anthropogenic ammonia emission inventory and its characteristics in 2013 [J]. Journal of Anhui Agricultural Sciences, 2015, 43 (29): 263–266 (in Chinese with English abstract).

    [48] Zhong L J, Zheng J Y, Louie P, et al. Quantitative uncertainty analysis in air pollutant emission inventories: methodology and case study [J]. Research of Environmental Sciences, 2007, 20 (4): 15–20 (in Chinese with English abstract).

This Article

ISSN:0250-3301

CN:11-1895/X

Vol 40, No. 11, Pages 4862-4869

November 2019

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Article Outline

Abstract

  • 1 Materials and methods
  • 2 Results and discussion
  • 3 Conclusions
  • References